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Wu, X.; Guo, J.; Sun, M.-Y.; Du, T.; Hao, D.-B.; Liu, D.; Wang, D.; Wen, S.; Yin, J.; Li, D.; He, J.* Construction of Heteroleptic Copper Complexes in Perylene Diimide-Based COFs for Heterogeneous Metallaphotoredox Catalysis. J. Am. Chem. Soc. accepted.